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Theoretical Study on Graphite and Lithium Metal as Anode Materials for Next-Gene

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ISBN-13
9789811389160
Type
NA
Publication Name
NA
ISBN
9789811389160
Publication Year
2024
Format
Trade Paperback
Language
English
Book Title
Theoretical Study on Graphite and Lithium Metal As Anode Materials for Next-Generation Rechargeable Batteries
Author
Gabin Yoon
Item Length
9.3in
Publisher
Springer
Genre
Technology & Engineering, Science
Topic
Materials Science / General, Chemistry / Physical & Theoretical, Nanotechnology & Mems, Power Resources / General
Item Width
6.1in
Item Weight
5 oz
Number of Pages
Xiv, 65 Pages

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Product Information

This thesis describes in-depth theoretical efforts to understand the reaction mechanism of graphite and lithium metal as anodes for next-generation rechargeable batteries. The first part deals with Na intercalation chemistry in graphite, whose understanding is crucial for utilizing graphite as an anode for Na-ion batteries. The author demonstrates that Na ion intercalation in graphite is thermodynamically unstable because of the unfavorable Na-graphene interaction. To address this issue, the inclusion of screening moieties, such as solvents, is suggested and proven to enable reversible Na-solvent cointercalation in graphite. Furthermore, the author provides the correlation between the intercalation behavior and the properties of solvents, suggesting a general strategy to tailor the electrochemical intercalation chemistry. The second part addresses the Li dendrite growth issue, which is preventing practical application of Li metal anodes. A continuum mechanics study considering various experimental conditions reveals the origins of irregular growth of Li metal. The findings provide crucial clues for developing effective counter strategies to control the Li metal growth, which will advance the application of high-energy-density Li metal anodes.

Product Identifiers

Publisher
Springer
ISBN-10
9811389160
ISBN-13
9789811389160
eBay Product ID (ePID)
17061244030

Product Key Features

Book Title
Theoretical Study on Graphite and Lithium Metal As Anode Materials for Next-Generation Rechargeable Batteries
Author
Gabin Yoon
Format
Trade Paperback
Language
English
Topic
Materials Science / General, Chemistry / Physical & Theoretical, Nanotechnology & Mems, Power Resources / General
Publication Year
2024
Genre
Technology & Engineering, Science
Number of Pages
Xiv, 65 Pages

Dimensions

Item Length
9.3in
Item Width
6.1in
Item Weight
5 oz

Additional Product Features

Number of Volumes
1 Vol.
Lc Classification Number
Qd551-578
Table of Content
1 Introduction.- 1.1 Demands for energy storage system.- 1.2 Li-ion batteries.- 1.3 Post Li-ion batteries.- 1.3.1 Na-ion batteries.- 1.3.2 Li metal batteries.- 1.4 References.- 2 Na intercalation chemistry in graphite.- 2.1 Introduction.- 2.2 Experimental and computational details.- 2.2.1 Materials.- 2.2.2 Electrode preparation and electrochemical measurements.- 2.2.3 Operando XRD analysis.- 2.2.4 Computational details.- 2.3 Staging behavior upon Na-solvent co-intercalation.- 2.4 Na-solvent co-intercalation into graphite structure.- 2.5 Solvent dependency on electrochemical properties.- 2.6 Conclusions.- 2.7 References.- 3 Conditions for reversible Na intercalation in graphite.- 3.1 Introduction.- 3.2 Computational details.- 3.3 Unstable Na intercalation in graphite.- 3.3.1 Destabilization energy of metal reconstruction.- 3.3.2 Destabilization energy of graphite framework upon intercalation.- 3.3.3 Local interaction between alkali metal ions and the graphite framework.- 3.3.4 Mitigating the unfavorable local interaction between Na and graphene layers.- 3.4 Conditions of solvents for reversible Na intercalation into graphite.- 3.4.1 Solvent dependency on reversible Na-solvent co-intercalation behavior.- 3.4.2 Thermodynamic stability of Na-solvent complex.- 3.4.3 Chemical stability of Na-solvent complex.- 3.4.4 Unified picture of Na-solvent co-intercalation behavior.- 3.5 Conclusions.- 3.6 References.- 4 Electrochemical deposition and stripping behavior of Li metal.- 4.1 Introduction.- 4.2 Computational details.- 4.3 Effect of deposition rate.- 4.4 Effect of surface geometry.- 4.5 Implications of SEI layer properties.- 4.6 Consequences of the history of deposition and stripping.- 4.7 Conclusions.- 4.8 References.
Copyright Date
2022
Dewey Decimal
621.3124240284
Series
Springer Theses Ser.
Dewey Edition
23
Illustrated
Yes

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